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PhD thesis, Waterford Institute of Technology. The initial part of this works involves the evaluation of a related series of bisamides for rational correlation between anion complexation and organocatalysis: remarkable enhancement of hydrogen bonding to anions was observed along with significant increases in catalytic activity in the Morita-Baylis-Hillman reaction. In addition, X-ray crystallography showed a large degree of pre-organisation was observed in one receptor by incorporation of bis trifluoromethyl aniline groups along with a thioamide functionality.
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