Organocatalysis thesis

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We use cookies to ensure that we give you the best experience on our website. By continuing to browse this repository, you give consent for essential cookies to be used. You can read more about our Privacy and Cookie Policy. Doctoral thesis, Durham University. We have studied the mechanism of the reaction of N-Boc imines and acetylacetone in the presence and absence of chiral phosphoric acid catalysts. In order to gain mechanistic insight into the asymmetric Mannich reaction, a structurally homologous series of N-Boc imines and BINOL-derived phosphoric acid and thiophosphoric acid catalysts were synthesised.
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PhD thesis, Waterford Institute of Technology. The initial part of this works involves the evaluation of a related series of bisamides for rational correlation between anion complexation and organocatalysis: remarkable enhancement of hydrogen bonding to anions was observed along with significant increases in catalytic activity in the Morita-Baylis-Hillman reaction. In addition, X-ray crystallography showed a large degree of pre-organisation was observed in one receptor by incorporation of bis trifluoromethyl aniline groups along with a thioamide functionality.
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Items in Dataspace are protected by copyright, with all rights reserved, unless otherwise indicated. Princeton University Doctoral Dissertations, Chemistry. Show full item record. All of DataSpace This Collection.
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